孙传智

发布时间:2024年02月23日 11:01 点击: 来源:






 

姓名孙传智

职称:

教授

专业:

物理化学/材料与化工,研究方向:能源、环境催化

导:

博导

最终学历:

博士

联系电话


电子邮件:

suncz@sdnu.edu.cn

简历及研究领域

个人简介

2011年博士毕业于南京大学化学化工37000cm威尼斯。西班牙国家研究委员会(CSIC)-瓦伦西亚理工大学(UPV)化学技术研究所(ITQ)访问学者。中国化工学会稀土催化与过程专业委员会委员,中国稀土学会催化专业委员会委员,期刊《Advanced Powder Materials》青年编委,山东师范大学“东岳学者”拔尖人才。

能源与环境问题是当今世界聚焦的热点问题。本课题组采用实验结合计算化学的研究方法从事相关领域的研究工作。第一,针对于火电厂及重型柴油车的烟气污染,主要聚焦于NOx的污染,研发新型负载型稀土基催化剂,克服现有催化剂有毒,高温稳定性差,低温活性低的缺陷。这不论在基础研究还是应用研究领域都具有十分重要的意义。第二,针对于目前国际热点能源问题——光水解制氢,展开研究工作。能源问题是人类目前面对的严峻问题,化石能源终将枯竭,人类开发替代能源刻不容缓。利用太阳光,在催化剂的作用下使水分解为氢气和氧气,这样,氢气可以成为人类取之不尽的燃料,若人类在此方向研究成功将具有划时代的意义。

欢迎有兴趣致力于能源与环境领域研究的同学加盟本课题组!


代表性论文

1. Xiaolin Xu, Xueqing Liu, Longfei Ma, Nana Liang, Shan Yang, Hao Liu, Jingfang Sun, Fang Huang,* Chuanzhi Sun,* and Lin Dong, Construction of Surface Synergetic Oxygen Vacancies on CuMn2O4 Spinel for Enhancing NO Reduction with CO, ACS Catal., 2024, 14, 30283040.

2. Menghan Gan, Shanshan Lai, Shujuan Jiang,* Chuanzhi Sun,* Shaoqing Song,* Dynamical transfer behavior and in situ interaction with H2O molecules of charge carriers over heterojunction in non-adiabatic systems, Appl. Catal. B: Environ., 2024, 340, 123278.

3. Yansong Wang, Shujuan Jiang,* Chuanzhi Sun,* Shaoqing Song,* Synchronously regulating d- and p-band centers of heterojunction photocatalysts by strain effect for solar energy conversion into H2, J. Mater. Sci.Technol., 2024, 190, 210-217.

4. Haitao Sun, Xueqing Liu, Yafeng Li, Fang Zhang, Xiuxiu Huang, Chuanzhi Sun,* and Fang Huang,* Mechanistic insights of electrocatalytic CO2 reduction by Mn complexes: synergistic effects of the ligands, Dalton Trans., 2024, 53, 1663.

5. Jie Wang, Yiqi Zhang, Shujuan Jiang,* Chuanzhi Sun,* and Shaoqing Song,* Regulation of d-Band Centers in Localized CdS Homojunctions through Facet Control for Improved Photocatalytic Water Splitting, Angew. Chem. Int. Ed., 2023, 62, e202307808.

6. Ke Liu, Shan Yang, Wei Li, Yifan Wang, Chuanzhi Sun,* Lu Peng,* Hermenegildo Garcia,* Non-noble-metal NiS promoted charge separation and photocatalytic hydrogen evolution for ZnCdS nano-islands on spherical SiO2, Fuel, 2023, 337, 126840.

7. Lijun Cheng, Songil Sin, Jiawei Ji, Shan Yang, Chong Tan, Zhiwen Gu, Wang Song, Chunkai Huang, Chuanzhi Sun,* Changjin Tang,* Lin Dong, Selective catalytic reduction of NO with NH3 over MnOx-CeO2 catalysts: The great synergy between CeO2 and crystalline phase of Mn3O4, Fuel, 2023, 342, 127772.

8. Shan Yang, Xinyu Guo, Ke Liu, Yafeng Li, Ting Li, Xianrui Gu, Raul Arenal, Xiaoxue Zheng, Wei Li, Chuanzhi Sun,* Houpeng Wang,* and Fang Huang,* Size effect of CoS2 cocatalyst on photocatalytic hydrogen evolutionperformance of g-C3N4, J. Colloid Interf. Sci., 2023, 635, 305-315.

9. Lijun Hu, Jiaqi Huang, Jie Wang, Shujuan Jiang,* Chuanzhi Sun,* Shaoqing Song,* Efficiently photocatalytic H2O overall splitting within the strengthened polarized field by reassembling surface single atoms, Appl. Catal. B: Environ., 2023, 320, 121945.

10. Jie Wang, Shujuan Jiang,* Chuanzhi Sun,* Shaoqing Song,* Delocalized ferroelectric engineering of efficient photo-generated charge directional transfer for solar energy conversion into H2, Chem. Eng. J., 2023, 452, 139468.

11. Songzhu Wang, Shan Yang, Shujuan Jiang, Chuanzhi Sun, Shaoqing Song,* Heterojunction within dual electric fields dynamically tailoring charge transfer to surface redox active sites for efficient H2 generation, Applied Surface Science, 2023, 612, 155847.

12. Fengzhou Chen, Jie Wang, Shan Yang, Shujuan Jiang,* Chuanzhi Sun,* and Shaoqing Song,* Activating Main-Group Mg Atomic Sites within Tri-s-triazine for Photocatalytic H2O Overall Splitting: Dynamic Mechanism and Performance, ACS Catal., 2023, 13, 5678-5688.

13. Jing Qiu, Yuanxiao Wu, Shujuan Jiang,* Chuanzhi Sun,* and Shaoqing Song,* Tuning p-Band Center of Carbon Nitride Homojunction Photocatalysts through Strain Effect for Solar-Driven H2 Production, ACS Energy Lett., 2023, 8, 4173-4178.

14. Wei Chen, Shan Yang, Hao Liu, Fang Huang, Qinghao, Lichen Liu,* Jingfang Sun, Chuanzhi Sun,* Dezhan Chen, and Lin Dong, Single-Atom Ce-Modified αFe2O3 for Selective Catalytic Reduction of NO with NH3, Environ. Sci. Technol. 2022, 56, 1044210453.

15. Jiaqi Huang, Shan Yang, Shujuan Jiang,* Chuanzhi Sun,* and Shaoqing Song,* Entropy-Increasing Single-Atom Photocatalysts Strengthening the Polarization Field for Boosting H2O Overall Splitting into H2, ACS Catal., 2022, 12, 14708-14716.

16. Yu Zhang, Shan Yang, Xiaoyue Zhu, Xiaolin Xu, Fang Huang*, Zhongnian Yang*, Chuanzhi Sun*, Effects of sulfation on hematite for selective catalytic reduction of nitrogen oxides with ammonia, J. Colloid Interf. Sci. 2022, 606, 1445-1456.

17. Guojian Yao, Shan Yang, Shujuan Jiang*, Chuanzhi Sun*, Shaoqing Song*, Spin polarized graphene monolayer of van der Waals heterojunction for photocatalytic H2O overall splitting, Appl. Catal. B: Environ., 2022, 315, 121569.

18. Jiari He, Lijun Hu, Chengtian Shao, Shujuan Jiang,* Chuanzhi Sun,* and Shaoqing Song*, Photocatalytic H2O Overall Splitting into H2 Bubbles by Single Atomic Sulfur Vacancy CdS with Spin Polarization Electric Field, ACS Nano 2021, 15, 1800618013.

19. Dongmei Tang, Chengtian Shao, Shujuan Jiang*, Chuanzhi Sun*, and Shaoqing Song*, Graphitic C2N3: An Allotrope of gC3N4 Containing Active Azide Pentagons as Metal-Free Photocatalyst for Abundant H2 Bubble Evolution, ACS Nano 2021, 15, 72087215.

20. Guojian Yao, Shan Yang, Jiari He, Shujuan Jiang*, Chuanzhi Sun*, Shaoqing Song*, In situ growing graphene on g-C3N4 with barrier-free interface and polarization electric field for strongly boosting solar energy conversion into H2 energy, Appl. Catal. B: Environ., 2021, 287, 119986.

21. Ke Liu, Lu Peng, Pingping Zhen, Lichao Chen, Shaoqing Song, Hermenegildo Garcia,*and Chuanzhi Sun*, ZnCdS Dotted with Highly Dispersed Pt Supported on SiO2 Nanospheres Promoting Photocatalytic Hydrogen Evolution, J. Phys. Chem. C 2021, 125, 14656−14665.

22. Yiming Zhou, Mohamed Elchalakani, et al, Chuanzhi Sun *Cleaning up oil pollution in the ocean with photocatalytic concrete marine structuresJ. Clean. Prod. 2021, 329, 129636

23. Yan Zhao, Shan Yang, Chengtian Shao, Shujuan Jiang*, Chuanzhi Sun*, Shaoqing Song*, Boosting charge spatial separation efficiency for catalytic H2 bubble evolution under macroscopic spontaneous polarization electric fieldChem. Eng. J. 2021, 421, 127812.

24. Chuanzhi Sun*, Wei Chen, Xuanxuan Jia, Annai Liu, Fei Gao, Shuai Feng*, Lin Dong*, Comprehensive understanding of the superior performance of Sm-modified Fe2O3 catalysts with regard to NO conversion and H2O/SO2 resistance in the NH3-SCR reaction, Chinese. J. Catal., 2021, 42, 417-430.

25. Xuanxuan Jia, Hao Liu, Yu Zhang, Wei Chen, Qing Tong, Guangxia Piao, Chuanzhi Sun*, Lin Dong, Understanding the high performance of an iron-antimony binary metal oxide catalyst in selective catalytic reduction of nitric oxide with ammonia and its tolerance of water/sulfur dioxide, J. Colloid Interf. Sci., 2021, 581, 427-441.

26. Lijun Hu1, Shan Yang1, Yan Zhao, Jiari He, Shujuan Jiang*, Chuanzhi Sun*, Shaoqing Song*, Spontaneous polarization electric field briskly boosting charge separation and transfer for sustainable photocatalytic H2 bubble evolutionAppl. Catal. B: Environ., 2021, 283, 119631.

27. Jinhua Luo, Jiari He, Shujuan Jiang*, Chuanzhi Sun*, Shaoqing Song*, In-plane coupling electric field driving charge directional transfer for highly efficient H2 bubble evolution, Chem. Eng. J. 2020, 396, 125365

28. Zhexing Lin, Chengtian Shao, Shujuan Jiang*, Chuanzhi Sun*, Shaoqing Song*, Hollow graphene with apparent potential difference to boost charge directional transfer for photocatalytic H2 evolution, Appl. Catal. B: Environ., 2020, 268, 118742.

29. Dan Zhang, Lu Peng, Ke Liu, Hermenegildo Garcia*, Chuanzhi Sun*, Lin Dong, Cobalt nanoparticle with tunable size supported on nitrogen-deficient graphitic carbon nitride for efficient visible light driven H2 evolution reaction, Chem. Eng. J. 2020, 381, 122576

30. Zhexing Lin, Yan Zhao, Jinhua Luo, Shujuan Jiang*, Chuanzhi Sun*, Shaoqing Song*, Apparent Potential Difference Boosting Directional Electron Transfer for Full Solar Spectrum‐Irradiated Catalytic H2 Evolution, Adv. Funct. Mater., 2019, 30, 1908797

31. Xiaoxue Zheng, Ke Liu, Lichao Chen, Hengxiao He, Lusheng Chen*, Chuanzhi Sun*, Co(O)x Particles in Polymeric N-Doped Carbon Nanotube Applied for Photocatalytic H2 or Electrocatalytic O2 Evolution, Polymers, 2019, 11(11), 1836

32. Hao Liu, Zhongxuan Fan, Chuanzhi Sun*, Shuohan Yu, Shuai Feng, Wei Chen, Dezhan Chen, Changjin Tang, Fei Gao, Lin Dong*, Improved activity and significant SO2 tolerance of samarium modified CeO2-TiO2 catalyst for NO selective catalytic reduction with NH3, Appl. Catal. B: Environ., 2019, 244, 671-683.

33. Hao Liu, Chuanzhi Sun*, Zhongxuan Fan, XuanXuan Jia, Jingfang Sun, Fei Gao, Changjin Tang, Lin Dong*, Doping effect of Sm on the TiO2/CeSmOx catalyst in the NH3-SCR reaction: structure–activity relationship, reaction mechanism and SO2 tolerance, Catal. Sci. Technol., 2019, 9, 3554–3567.

34. Chuanzhi Sun*, Hui Zhang, Hao Liu, Xiaoxue Zheng, Weixin Zou, Lin Dong*, Lei Qi, Enhanced activity of visible-light photocatalytic H2 evolution of sulfur doped g-C3N4 photocatalyst via nanoparticle metal Ni as cocatalyst, Appl. Catal. B: Environ., 2018, 235, 66-74.

35. Chuanzhi Sun*, Hao Liu, Wei Chen, Dezhan Chen, Shuohan Yu, Annai Liu, Lin Dong*, Shuai Feng, Insights into the Sm/Zr co-doping effects on N2 selectivity and SO2 resistance of a MnOx-TiO2 catalyst for the NH3-SCR reaction, Chem. Eng. J., 2018, 347, 27-40.

36. Shaoqing Song, Changhai Lu, Xi Wu, Shujuan Jiang*, Chuanzhi Sun*, Zhanggao Le*, Strong base g-C3N4 with perfect structure for photocatalytically eliminating formaldehyde under visible-light irradiation, Appl. Catal. B: Environ., 2018, 227, 145-152.

37. Xi Wu, Shujuan Jiang, Shaoqing Song*, Chuanzhi Sun*, Constructing effective photocatalytic purification system with P-introduced g-C3N4 for elimination of UO22+, Applied Surface Science, 2018, 205, 319-32

38. Xi Wu, Changhai Lu, Jingjie Liu, Shaoqing Song*, Chuanzhi Sun*, Constructing efficient solar light photocatalytic system with Ag-introduced carbon nitride for organic pollutant elimination, Appl. Catal. B: Environ., 2017, 217, 232-240.

39. Lin Ke, Peifeng Li, Xi Wu, Shujuan Jiang*, Mingbiao Luo, Yunhai Liu*, Zhanggao Le, Chuanzhi Sun*, Shaoqing Song*, Graphene-like sulfur-doped g-C3N4 for photocatalytic reduction elimination of UO22+ under visible Light, Appl. Catal. B: Environ., 2017, 205, 319-326.

40. Weixi Fan, Chuanzhi Sun*, Fang Huang, Jianbiao Liu, Xue Zhao, Xiehuang Sheng and Dezhan Chen*, Mechanistic insight into the regioselectivity of Pd(II)-catalyzed C–H functionalization of N-methoxy cinnamamide, Dalton Trans., 2017, 46, 5288-5296.

41. Chuanzhi Sun, Yingjie Tang, Fei Gao, Jingfang Sun, Kaili Ma, Changjin Tang and Lin Dong*, Effects of different manganese precursors as promoters on catalytic performance of CuO–MnOx/TiO2 catalysts for NO removal by CO, Phys.Chem.Chem.Phys., 2015, 17, 15996-16006.

42. Chuanzhi Sun, Mingshu Liu, Haitao Sun, Fang Huang, Nan Sun, Dezhan Chen*, Theoretical mechanism for selective catalysis of ruthenium complex catalyzed hydroboration of terminal alkynes to Z-vinylboronates, Inter. J. Quantum Chem., 2015,115, 59-67.

43. Xue Zhao, Chuanzhi Sun*, Yating Lu, Zhong Xing, Nan Sun, Dezhan Chen*, A DFT study on the difference of C–H bond activation by Pd(II) and Pd(IV) complex, Comput. Theor. Chem., 2015, 1056, 41-46.

44. Mingshu Liu, Chuanzhi Sun*, Fang Huang, Nan Sun, Dezhan Chen*, Theoretical mechanism for selective catalysis of double hydrophosphination of terminal arylacetylenes by an iron complex, Dalton Trans., 2014, 43, 4813-4821.

45. Chuanzhi Sun, Kui Wang, Haitao Sun, Nan Sun, Dezhan Chen*, A DFT study on a muti-pathways, one product reaction: initially divergent radical reactions reconverge to form a single product, Inter. J. Quantum Chem., 2014, 114, 769-781.

46. Chuanzhi Sun, Xiaodan He, Wenjuan Wang, Guohong Chu, Shuxiang Zhang, Dezhan Chen*, Computational study on the mechanism of uncatalyzed and selenium-based catalyzed bromolactonization, Comput. Theor. Chem., 2014,1046, 49-56.

47. Jinfeng Zhao, Chuanzhi Sun*, Nan Sun, Lin Meng, Dezhan Chen*, Theoretical study on the mechanism of the reaction for alkene hydroaminations catalyzed by chiral aldehyde, Inter. J. Quantum Chem., 2013, 113, 2457-2463.

48. Linlin Cao, Chuanzhi Sun*, Nan Sun, Lin Meng, Dezhan Chen*, Theoretical mechanism studies on the electrocatalytic reduction of CO2 to formate by water-stable iridium dihydride pincer complex, Dalton Trans., 2013,42, 5755-5763.

49. Chuanzhi Sun, Jie Zhu, Yuanyuan Lv, Lei Qi, Bin Liu, Fei Gao, Keqin Sun, Lin Dong*, Yi Chen, Dispersion, reduction and catalytic performance of CuO supported on ZrO2-doped TiO2 for NO removal by CO, Appl. Catal. B: Environ., 2011, 103, 206-220.

50. Chuanzhi Sun, Lihui Dong, Wujiang Yu, Lichen Liu, Hao Li, Fei Gao*, Lin Dong*, Yi Chen, Promotion effect of tungsten oxide on SCR of NO with NH3 for the V2O5-WO3/Ti0.5Sn0.5O2 catalyst: Experiments combined with DFT calculations, J. Mol. Catal. A: Chem., 2011, 346, 29-38.

51. Chuanzhi Sun, Lichen Liu, Lei Qi, Hao Li, Hongliang Zhang, Changshun Li, Fei Gao*, Lin Dong*, Efficient fabrication of ZrO2-doped TiO2 hollow nanospheres with enhanced photocatalytic activity of rhodamine B degradation, J. colloid Interf. Sci., 2011, 364, 288-297.

研究课题

国家自然科学基金面上项目22372093

稀土改性铁基催化剂表面受阻路易斯酸碱对协同脱硝作用机制研究

国家自然科学基金面上项目21976111

稀土掺杂金属氧化物脱硝催化剂的创制及其抗硫中毒机制的原位技术研究

山东省自然科学基金面上项目ZR2019MB052

稀土掺杂金属氧化物催化剂在NOx消除中的应用及其抗硫中毒机制原位技术研

国家自然科学基金青年项目21403134

暴露晶面可控的CexM1-xO2M=Ti,ZrHf)固溶体制备及其在NOx催化消除中的作用机制  

山东省科技攻关项目 2014GGX102019

基于铈基固溶体的暴露晶面控制及其在脱硝催化剂中的应用

荣誉称号

20141

山东师范大学教学成果奖(三等奖)

20179

山东师范大学优秀教学奖

201811

山东师范大学研究生“五导”卓越导学团队荣誉称号

20207

山东师范大学科研创新团队带头人

20223

山东省第九届教学成果奖(一等奖)

20239

山东师范大学“十佳教师”